两束啁啾脉冲控制下的H+D~+光缔合反应研究
Photoassociation reaction of H+D~+ in two chirped pulses
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摘要: 从理论上研究了两束啁啾脉冲控制H+D+的光缔合反应.第一束脉冲用来加速碰撞伴的碰撞速度,第二束脉冲用来增加产物HD+的产率.结果表明:第一束脉冲的参数决定了第二束脉冲的优化参数以及产物HD+的布居.产物的布居可以通过调节两束脉冲的延迟时间得到控制.Abstract: The photoassociation reaction H+D+ induced by two chirped pulses is theoretically studied.The first pulse is employed to accelerate the collision pairs,and the second pulse is used to enhance the yield ratio of HD+.The optimal parameters of the second pulse and the population of product HD+ depend on the chirp rate of the first pulse.The population of the product HD+ can be controlled by the delay time between the two laser pulses.
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